Entanglement is an intrinsic property of quantum mechanics and its measurement probes the current understanding of the underlying quantum nature of elementary particles at a fundamental level. A measurement of the extent of entanglement in top quark-antiquark ($\mathrm{t\bar{t}}$) events produced in proton-proton collisions at a center-of-mass energy of 13 TeV is performed on the data recorded by the CMS experiment at the CERN LHC in 2016, corresponding to an integrated luminosity of 35.9 $\mathrm{fb^{-1}}$. The events are selected based on the presence of two oppositely charged high transverse momentum leptons. An entanglement-sensitive observable $D$ is derived from the top quark spin-dependent parts of the $\mathrm{t\bar{t}}$ production density matrix. Values of $D$ smaller than $-1/3$ are evidence of entanglement and, within a particular phase space, $D$ is measured to be $-0.478^{+0.025}_{-0.027}$. With an expected (observed) significance of 5.1 (5.7) standard deviations, this provides observation for quantum mechanical entanglement within $\mathrm{t\bar{t}}$ pairs in this phase space. This measurement provides a new quantum probe of the inner workings of the standard model at the highest energy ever tested.
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